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© Research
Publication : The journal of physical chemistry. B

Thermal diffusion and molecular diffusion values for some alkane mixtures: a comparison between thermogravitational column and thermal diffusion forced rayleigh scattering

Scientific Fields
Diseases
Organisms
Applications
Technique

Published in The journal of physical chemistry. B - 21 Jun 2008

Blanco P, Polyakov P, Bou-Ali MM, Wiegand S

Link to Pubmed [PMID] – 18570400

J Phys Chem B 2008 Jul;112(28):8340-5

In the present work we studied the thermal diffusion behavior of n-decane in various alkanes by thermogravitational column (TC) technique and the thermal diffusion forced Rayleigh scattering (TDFRS) method. The investigated lighter alkanes compared to n-decane are n-pentane, n-hexane, n-heptane, n-octane, and the heavier ones are n-tetradecane, n-pentadecane, n-hexadecane, n-heptadecane, n-octadecane, and n-eicosane. The binary mixture n-decane/ n-pentane we investigated at several different concentrations; all other mixtures were only investigated at a mass fraction of 50%. Even for the volatile n-pentane/ n-decane mixture the deviations between the thermal diffusion coefficients determined by the different methods agreed within the error bars. Typically the agreement between the two methods was in the order of 5%. In comparison to recently published TC and TDFRS data we found deviations in the order of 30% up to 40%. We analyze and discuss the possible reasons for the discrepancies for the present and the past publications.

http://www.ncbi.nlm.nih.gov/pubmed/18570400